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The Chromebook has a front-facing webcam, and this app takes good advantage of it. In addition to allowing snapshots from the camera, Webcam Toy also has a number of fun effects like the one shown here.
I use Evernote on every device I use, and this app makes it easy to do with Chrome.
I run it in a window on the Chromebook and use it to both capture information and write articles.
This app is a simple interface for Google Chat, allowing audio/video chat sessions with your contacts. Used in a separate window I keep it open on my Chromebook to the side of the screen.