@conflipper The only advantage to using x64 Office 2010 is if your Office programs actually need more than 4Gb of RAM each. Install the 32bit Office 2010 and you'll be fine on x64 Windows. Are you working with 4Gb Excel files?
Also, no Outlook x64 does not work with WMDC: http://pocketnow.com/thought/reminder-dont-install-64-bit-outlook-if-you-want-to-sync
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